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Session Overview
Session
TOM Ultrafast S3: Ultrafast Phenomena
Time:
Thursday, 28/Aug/2025:
10:30am - 12:00pm

Location: Commissiekamer 3


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Presentations
10:30am - 11:00am
INVITED

Lightwave-Controlled Relativistic Plasma Mirrors At kHz Repetition Rate

Antoine Cavagna1, Milo Eder2, Jaismeen Kaur1, André Kalouguine1, Christian Cabello1, Marie Ouillé1, Gérard Mourou3, Enam Chowdhury4, Stefan Haessler1, Rodrigo Lopez-Martens1

1Laboratoire d'Optique Appliquée (LOA), IP-Paris, CNRS, France; 2Department of Physics, The Ohio State University, USA; 3Ecole polytechnique, France; 4Department of Materials Science and Engineering, Fontana Laboratories, The Ohio State University, USA

Plasma mirrors driven at kHz-repetition-rate with waveform-controlled relativistic-intensity near-single-cycle laser pulses produce extreme ultraviolet spectral continua supporting isolated attosecond pulses with diffraction limited beam quality. A newly developed liquid leaf target yields unprecedented stability and duration of operation. This lifts a major obstacle to exploiting plasma mirrors as attosecond pulse sources.



11:00am - 11:15am

Boosting solid-state high-harmonic generation efficiency by non-collinear XUV wave mixing with two-color drivers

Nataliia Kuzkova1,2, Sylvianne D. C. Roscam Abbing1, Roy van der Linden1, Filippo Campi1, Brian de Keijzer1, Corentin Morice3, Zhuang-Yan Zhang1, Maarten L. S. van der Geest1, Peter M. Kraus1,2

1Advanced Research Institute for Nanolithography, The Netherlands; 2Vrije Universiteit, Department of Physics and Astronomy, The Netherlands; 3University of Amsterdam, Institute for Theoretical Physics, The Netherlands

We present studies on boosting high-harmonic generation (HHG) efficiency from solids in the extreme-ultraviolet (XUV) region by two-color non-collinear wave mixing in silica. Our results show that the conversion efficiency of two-color wave mixing exceeds that of single-color HHG by a factor of at least ten. We analyze the underlying mechanisms, revealing that the synergy between Floquet-Bloch dressing and inter- and intraband dynamics under laser irradiation enables efficient carrier excitation, enhancing harmonic yield. Integrating wave mixing into solid-state HHG could help establish compact, coherent XUV sources for applications where traditional gas-HHG is impractical.



11:15am - 11:30am

In-situ frequency comb shaping by multi-frequency injection in fast-gain lasers

Alexander Dikopoltsev, Diego Piciocchi, Ina Heckelmann, Bahareh Marzban, Lucius Miller, Mattias Beck, Giacomo Scalari, Jérôme Faist

ETH Zurich, Switzerland

Shaping of the spectrum of frequency comb sources is highly beneficial for application that require controllable optical source, such as ranging or communications. However, efficient in-situ reconfiguration of the spectrum is a challenge. We demonstrate spectral shaping of frequency combs in fast-gain active devices by engineering an Aharonov-Bohm phase in a synthetic frequency lattice. By modulating a fast gain circular laser at its resonance and twice this frequency with a relative phase, we created a triangular ladder in the modal space, where the phase added with staggered phase flux. This broke the time-reversal symmetry in the system, allowing for non-trivial gauge fields that manipulate the light. This enable the control over the frequency lattice dynamics, enabling full bandwidth tuning of a strong central lobe in a Quantum Cascade Laser comb. This paves the wave to new efficient and simple reconfigurable optical frequency comb sources.



11:30am - 11:45am

Conservation laws of generalized angular momentum by second-harmonic generation in underdense plasmas

Alexis Voisine1, Pierre Béjot1, Franck Billard1, Hugo Marroux2, Olivier Faucher1, Edouard Hertz1

1ICB, UMR CNRS 6303 - Université Bourgogne Europe, Dijon, 21078, France; 2Université Paris-Saclay CEA,CNRS LIDYL Gif-sur-Yvette 91191, France

Light beams exhibit two intrinsic quantized degrees of freedom: spin angular momentum (SAM) and orbital angular momentum (OAM) whose manipulation enables precise control over the topological characteristics of electromagnetic fields. Recently, structured fields formed from a non-separable combination of SAM and OAM have attracted significant interest. These fields correspond to eigenstates of the generalized angular momentum (GAM), an operator merging SAM and OAM components which can yield remarkable fractional eigenvalues. The conservation of GAM, observed through harmonic generation, suggests its potential significance as a fundamental quantum number. In this work, we extend the analysis by examining its conservation laws through second-harmonic generation within an underdense, isotropic, and inhomogeneous plasma; a process governed by dipole-forbidden interaction which implies spin-orbit coupling. Our findings indicate that the symmetry and topological properties of the field are disrupted, leading to conservation of the GAM charge only on average. This symmetry breaking provides an easily detectable signature of the driving field’s topology



 
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