Quantum technologies require advanced optical metamaterials whose properties can be tailored and controlled as desired. Hyperbolic metamaterials have great potential for applications in nonlinear nanophotonics, such as all-optical switching, optical limiting, mode-locking and optical sensing. In this work, we show how to obtain strong third-order optical nonlinearities in hyperbolic multilayers exploiting the effect of bulk plasmon polaritons. We demonstrate the tunability of these properties with angle and polarization, and we propose a model to predict them. We evidence the enhancement of the nonlinear response in low-loss metamaterials.

We report that Ca3TaAl3Si2O14 is a positive uniaxial crystal and provides second-order frequency conversion. Indeed, we performed direct measurements of phase-matching conditions for second-harmonic generation and sum-frequency generation up to 3.5 µm. The simultaneous fitting of recorded data provided the Sellmeier equations of the two principal refractive indices and the magnitude of the nonlinear coefficient.

We report a new and more precise Sellmeier equation derived using the quasi-phase-matching curves obtained from the study of the optical parametric generation (OPG) in 1D periodically poled LiTaO3 (1D-PPLT) of different periods at low and high pump power

Photon energy upconversion, i.e. the conversion of several low-energy photons to a photon of higher energy, offers significant potential for nano-optoelectronics and nanophotonics applications. The primary challenge is to achieve high upconversion efficiency and a broad device performance range, enabling effective upconversion even at low excitation power. This study demonstrates that core/shell semiconductor nanowire heterostructures can exhibit upconversion efficiencies exceeding what was previously reported for semiconductor nanostructures even at a low excitation power of 100 mW/cm2, by a two-photon absorption process through conduction band states of the narrow-bandgap nanowire shell region. By engineering the electric-field distribution of the excitation light inside the NWs, upconversion efficiency can be further improved by eight times. This work showcases the effectiveness of the proposed approach in achieving efficient photon upconversion using core/shell NW heterostructures, resulting in some of the highest upconversion efficiencies reported in semiconductor nanostructures. Additionally, it offers design guidelines for enhancing energy upconversion efficiency.

We built and studied a singly resonant optical parametric oscillator using a 5%MgO:PPLN partial cylinder pumped by a sub-nanosecond microlaser emitting 1064 nm at a repetition rate of 1kHz. It is continuously tunable from 1410 nm up to 4330 nm by rotating the cylinder and a total energy of several micro Joules is emitted with a beam quality factor M² lower than 3.