Thin-disk laser oscillators can nowadays reach few tens of femtosecond pulses at gigawatt-level intracavity powers and megahertz-repetition rates becoming increasingly more powerful sources for intra-oscillator high harmonic generation (HHG). Currently, we can generate high harmonics in neon reaching photon energies of 70 eV, which we expect to increase toward 100 eV in the near future. In parallel, the achievable average and peak output powers of these oscillators in the range of 100 W and 100 MW, respectively, make these sources very promising to drive HHG in single-pass configuration after nonlinear pulse compression. Starting from transform-limited 30 to 50-fs soliton output soliton pulses of TDL oscillators, we will likely see these lasers approaching a single-cycle regime becoming highly attractive sources for attosecond science.

We present a table-top, efficient and power scalable scheme enabling the effective generation of extreme ultraviolet radiation up to 100 eV photon energy. Therefor ultrashort pulses (< 20fs) in the visible spectral range (515 nm) are used to drive high harmonic generation in helium. This allows for a significant efficiency boost compared to near-infrared (NIR) drivers, enabled by the favourable scaling of the single-atom response of λ-6 [1]. The experimental realization of a mulitpass cell delivering 15.7 fs pulses with a peak power close to 25 GW at 515 nm and an overall efficiency (IR to compressed green pulse) of >40 %. In conjunction, preliminary HHG results will be presented, paving the way for mW-class HHG sources at 13.5 nm.

The technological refinements on high-power laser systems of Petawatt class unveil scenarios for light-matter interaction beyond the laser-plasma perspective. In this contribution we explore the possibility of assisting high-harmonic generation (HHG) with the strong magnetic field associated with one of those intense sources. Recently, there has been an interest in developing schemes to employ intense laser beams to define spatial volumes in which strong magnetic fields are found isolated from the electric field. In this conditions, the magnetic field can be used to assist the harmonic generation from atoms from standard drivers. We demonstrate that, using the proper interaction geometry, the magnetic field confines the transversal dynamics of the continuum electrons allowing, on one side, to enhance the efficiency of the electron rescattering that produces the harmonic radiation and, on the other side, to excite the electron transverse dynamics and to convert this energy into phase-locked harmonic photons of few hundreds of eV.

We report on a high energy ultrafast fibre laser architecture designed for high harmonics generation in solids. The laser delivering 50 fs pulses with 2.12 µJ at 1550 nm has enabled the generation of harmonics up to harmonic H5 from a magnesium oxide (MgO) bulk sample. To the best of our knowledge this is the first solid-state HHG source driven by a µJ-class few-cycle fiber laser in the mid-IR region.

A phase-matching free pulse retrieval technique based on plasma-induced defocusing in a rare gas is presented. Based on a pump-probe setup, this technique uses a moderately intense pump laser pulse for ionizing the medium, creating in turn an ultrafast defocusing lens. While a coronagraph blocks out the probe pulse in absence of ionization, the plasma lens leads to increase the probe beam size in the far field. By measuring the spectrum of the probe propagating around the coronagraph as a function of the pump-probe delay t, a bi-dimensional trace (w-t) is obtained. This enables to fully characterize the temporal and spectral characteristics of the probe pulse through a method that is free of phase matching constraints. Demonstrated both in the near-infrared (800 nm) and in the ultraviolet (266 nm), the present technique is potentially suited for characterizing pulses in the whole transparency region of the used gas, i.e., from the deep-ultraviolet to the far-infrared.

We point out the breakdown of two approximations widely used to describe decoherence in open quantum systems, the secular and Markov approximations. We probe their limits by studying the influence of pressure on the alignment revivals (echoes) created in properly chosen gas mixtures (HCl and CO2, pure and diluted in He) by one (two) intense and short laser pulse(s). Experiments, as well as predictions using molecular dynamics simulations, consistently demonstrate in some of the aforementioned systems the break-down of these approximations at very short times (<15 ps) after the laser kick(s).