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Session Overview
Location: Meursault/ Nuit ST-G./Corton
Date: Tuesday, 12/Sept/2023
10:30am - 12:00pmTOM5 S01: Nanomaterials and applications
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Azzedine Boudrioua, LPL, Université Sorbonne Paris Nord, France
 
10:30am - 11:00am
Invited
ID: 278 / TOM5 S01: 1
TOM 5 Optical Materials

Asymmetric dual-grating-gate plasmonic THz detectors based on InGaAs-channel HEMT and graphene-channel FET

Akira Satou, Taiichi Otsuji

Research Institute of Electrical Communication, Tohoku University, Japan

Towards realization of beyond-5G large-capacity and ultrahigh-speed terahertz (THz) wireless communication systems, we have developed InGaAs-channel high-electron-mobility transistor (HEMT) and graphene-channel field-effect transistor (G-FET) plasmonic THz detectors, featured by original asymmetric dual-grating-gate (A-DGG) structures. The A-DGG fingers act as a broadband deep-subwavelength grating coupler that converts incoming THz waves into 2D plasmons in the channel, and their strong hydrodynamic nonlinearities as well as their fast response enable fast, highly sensitive THz detection at room temperature.

In this talk, we review recent advances of the A-DGG plasmonic THz detectors and demonstrate that they are promising for use in beyond-5G wireless communication systems. First, we investigate a new way to read out the photovoltage from the gate electrode of an A-DGG InGaAs-channel HEMT that enables the enhancement of responsivity in proportion to the active area size as well as the impedance matching to 50-Ω interconnection systems. Second, we demonstrate that a new plasmonic THz detection mechanism called “3D rectification effect” in an A-DGG InGaAs-channel HEMT in the gate-readout configuration drastically enhances the responsivity. Third, we reveal that, in an A-DGG G-FET, both plasmonic and photothermoelectric effects coexist as THz detection mechanisms, resulting in the high responsivity and 10-ps-order fast response time.



11:00am - 11:15am
ID: 152 / TOM5 S01: 2
TOM 5 Optical Materials

Controlling the strong light-matter coupling in metal-dielectric optical resonators using spin-crossover molecules

Karl Ridier1, Lijun Zhang1, Stéphane Calvez2, Lionel Salmon1, Gábor Molnár1, Azzedine Bousseksou1

1CNRS - Laboratoire de Chimie de Coordination, France; 2CNRS - Laboratoire d’Analyse et d’Architecture des Systèmes, France

We report the observation of (ultra)strong light-matter coupling, in the UV spectral region, between optical modes of a metal/dielectric bilayer nanocavity and the electronic excitations of spin-crossover (SCO) molecules. By thermally switching the SCO molecules between their low-spin and high-spin states, we demonstrate the possibility of fine-tuning the light-molecule hybridization strength, allowing a reversible switching between strong- (with Rabi splitting values of up to 550 meV) and weak-coupling regimes within a single photonic resonator. As a result, we show that spin-crossover molecular compounds constitute a novel, promising class of active nanomaterials in the context of tuneable and reconfigurable polaritonic devices.



11:15am - 11:30am
ID: 194 / TOM5 S01: 3
TOM 5 Optical Materials

Strong Er^3+ radiative emission enhancement by quasi-BIC modes coupling in all-dielectric slot nanoantenna arrays

Boris Kalinic1, Tiziana Cesca1, Mirko Trevisani1, Andrea Jacassi2, Riccardo Sapienza2, Giovanni Mattei1

1Dept. of Physics and Astronomy, University of Padova, Italy; 2The Blackett Laboratory, Dept. of Physics, Imperial College London, UK

We have designed and realized all-dielectric lossless nanoantennas, in which a thin SiO2 layer doped with erbium ions is placed inside slotted silicon nanopillars arranged in a square array. The modal analysis has evidenced that the slotted nanopillar array supports optical quasi-BIC resonances with ultra-high Q-factors (up to Q∼10^9), able to boost the electromagnetic local density of optical states in the optically active layer. Up to 3 orders of magnitude photoluminescence intensity increment and 2 orders of magnitude decay rate enhancement have been measured at room temperature when the Er^(3+) emission at about λ=1540 nm couples with the quasi-BIC resonances. Furthermore, by tailoring the nanopillar aspect ratio, the slot geometry has been exploited to obtain selective enhancements of the electric or magnetic dipole contribution to Er^(3+) radiative transitions in the NIR, keeping the emitter quantum efficiency almost unitary. Finally, by computing the angularly resolved electromagnetic field enhancement inside the nanoslot, the nanoantenna directivity has been designed, proving that strong beaming effects can be obtained. Our findings have a direct impact on the development of bright and efficient photon sources operating at telecom wavelength that are of primary importance for quantum nanophotonic applications.



11:30am - 11:45am
ID: 292 / TOM5 S01: 4
TOM 5 Optical Materials

Fabrication of nanometre sized gratings via ion irradiation

Johannes Michael Kaufmann1, Frank Schrempel1, Uwe Zeitner2

1Institute of Applied Physics Friedrich Schiller University Jena; 2Fraunhofer Institute for Applied Optics and Precision Engineering

The damage caused by irradiation of crystalline material with ions results in localized volume changes. Here, swelling is utilized to fabricate nanostructured gratings with heights below 10 nm for extreme ultraviolet radiation. Irradiations were performed through a structured layer of photoresist shadowing parts of the sample from a broad ion beam. This enabled much shorter fabrication times than comparable direct write processes with a focussed ion beam. The study presents results from first systematic investigations regarding the fabrication of nanostructured gratings by irradiation of silicon with a broad beam of helium ions with energies of 30 keV. A smaller, scanned beam is used for comparison. Fluence was varied from 0.4 to 7.5×1e16 ions/cm^2 . Fabricated structures were measured via atomic force microscopy. This yielded a controllable method to fabricate shallow gratings with heights in the range of 0 to 10 nm.



11:45am - 12:00pm
ID: 417 / TOM5 S01: 5
TOM 5 Optical Materials

Optical control of hierarchical DNA-functionalized nanoparticle self-assembly on 2D surfaces

Talha Erdem, Zeynep Şenel, Ruby Phul, Akrema Akrema, Ahmet Faruk Yazıcı, Emirhan Taze, Evren Mutlugün

ABDULLAH GÜL UNIVERSITY, Turkiye

We investigated the effect of light on the DNA-driven self-assembly to form hierarchical patterns on two dimensional surfaces. We specifically focused on the self-assembly of DNA-functionalized quantum dots (QDs) onto DNA-functionalized glass substrate while illuminating the surface with a laser during coating process. The region illuminated with a green laser remained uncoated with red-emitting QDs while the not-illuminated region was successfully coated. Next, a red laser whose light cannot be absorbed by the red-emitting QDs did not avoid the DNA-driven self-assembly of the QDs onto glass substrate. Additionally, we demonstrated that silica nanoparticles that had been functionalized with DNA and are not able to absorb the light in the visible regime were again coated on the surface while being exposed to a green laser. These results prove that the absorption of the light is responsible for controlling the binding-unbinding process of QDs. Finally, we added DNA-functionalized green-emitting QDs onto the area that was not coated with red-emitting QDs under the green laser exposure. We observed successful coating of previously uncoated regions with the green QDs. This revealed the viability of our technique for building up hierarchical structures without using, sophisticated, or resource-intensive microfabrication methods.

 
1:30pm - 3:00pmTOM5 S02: Optical materials and devices
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Tiziana Cesca, University of Padova, Italy
 
1:30pm - 2:00pm
Invited
ID: 226 / TOM5 S02: 1
TOM 5 Optical Materials

Exploiting the natural instability in thin and flexible dielectric solid films for sensing and photonic applications

Nicoletta Granchi1, Luca Fagiani2, Chiara Barri2, Mehrnaz Modaresialam3, Michele Gherardi2, Angelo gatta Zini2, Benedetta Maria Squeo4, Mariacecilia Pasini4, Andrea Chiappini5, Laura Pasquardini6, Alexey Fedorov7, Marco Abbarchi8, Maria Antonietta Vincenti9, Francesca Intonti1, Monica Bollani7

1LENS and Department of Physics and Astronomy, University of Florence, Italy; 2Department of Physics, Politecnico di Milano, Milano, Italy; 3Aix Marseille Univ, Université de Toulon, CNRS, IM2NP Marseille, France; 4Institute of Chemical Sciences and Technologies (SCITEC) – CNR, Milano, Italy; 5Institute of Photonics and Nanotechnology (IFN) – CNR, Trento, Italy; 6Indivenire srl, Trento, Italy; 7Institute of Photonic and Nanotechnology (IFN)- CNR, LNESS laboratory, Como, Italy; 8Solnil, 95 Rue de la République, Marseille, 13002, France; 9Department of Information Engineering, University of Brescia, Brescia, Italy

Flexible and stretchable photonics are emerging fields aiming to develop novel applications where the devices need to conform to uneven surfaces or whenever lightness and reduced thickness are major requirements. However, owing to the relatively small refractive index of transparent soft matter, these materials are not well adapted for light management at visible and near-infrared frequencies. Here we demonstrate simple, low cost and efficient protocols for fabricating Si1−xGex-based, sub-micrometric dielectric antennas with ensuing hybrid integration into different plastic supports. The dielectric antennas are realized exploiting the natural instability of thin solid films to form regular patterns of monocrystalline atomically smooth silicon and germanium nanostructures. Efficient protocols for encapsulating them into flexible and transparent, organic supports are investigated and validated. We benchmark the optical quality of the antennas with light scattering measurements, demonstrating the control of the islands structural colour and the onset of sharp Mie modes after encapsulation.



2:00pm - 2:15pm
ID: 315 / TOM5 S02: 2
TOM 5 Optical Materials

Fabrication and assessment of mechanically flexible 1D photonic crystals

Giacomo Zanetti1,4, Alice Carlotto1, Thi Ngoc Lam Tran1,2,3, Anna Szczurek5, Bartosz Babiarczuk5, Osman Sayginer6, Stefano Varas1, Justyna Krzak5, Oreste Bursi7,1, Daniele Zonta7,1, Anna Lukowiak8, Giancarlo Righini9, Maurizio Ferrari1, Giacomo Baldi4, Matteo Bonomo10, Simone Galliano10, Claudia Barolo10, Nicola Bazzanella11, Silvia Maria Pietralunga12, Alessandro Chiasera1

1IFN-CNR, CSMFO Lab. and FBK Photonics Unit, Via alla Cascata 56/C, 38123 Povo (TN), Italy; 2Dept. of Physics, Politecnico di Milano, P.zza L. da Vinci 32, 20133 Milan, Italy; 3Dept. of Materials Technology, Faculty of Applied Sciences, Ho Chi Minh City University of Technology and Education, Vo Van Ngan Str. 1, Thu Duc District, 720214 Ho Chi Minh City, Vietnam; 4Department of Physics, University of Trento, Via Sommarive 14, 38123 Povo (TN), Italy; 5Dept. of Mechanics, Materials and Biomedical Engineering, Wroclaw University of Science and Technology, Smoluchowskiego 25, Wroclaw, 50-370, Poland; 6Biological Imaging and TranslaTUM, Technische Universität München, Ismaninger Str. 22, Munich, D-81675, Germany; 7Dept. of Civil, Environmental and Mechanical Engineering, University of Trento, via Mesiano 77, Trento, 38123, Italy; 8Institute of Low Temperature and Structure Research, PAS, ul. Okólna 2, Wroclaw, 50422, Poland; 9National Research Council (CNR), Institute of Applied Physics (IFAC) “Nello Carrara”, Via Madonna del Piano 10, Florence, Sesto Fiorentino, 50019, Italy; 10Department of Chemistry, NIS Interdepartmental Centre and INSTM Reference Centre, University of Turin, Via Pietro Giuria 7, Turin, 10125, Italy; 11Laboratorio Idrogeno Energia Ambiente (IdEA), Department of Physics, University of Trento, Via Sommarive 14, 38123 Povo (TN), Italy; 12IFN-CNR, P.zza Leonardo da Vinci 32, Milan, 20133, Italy

Flexible glass photonics is a cutting-edge technological and scientific research field that, thanks to a very broad spectrum of applications, has tremendously grown during the last decade and is now a strategic topic. Here, we present the results of the spectral transmittance and reflectance of a 10-layer SiO2/TiO2 1D photonic crystal deposited on a flexible polymeric substrate under different bending conditions, obtained with a home-made adjustable sample holder.



2:15pm - 2:30pm
ID: 367 / TOM5 S02: 3
TOM 5 Optical Materials

Design and fabrication of a vanadium dioxide-based actively switchable wire grid polarizer for near-infrared applications

Markus Walther1, Thomas Siefke1,2, Kristin Gerold2, Uwe Detlef Zeitner2,3

1Friedrich Schiller University Jena, Germany; 2Fraunhofer Institute for Applied Optics and Precision Engineering IOF; 3Munich University of Applied Sciences

This study introduces an actively switchable wire grid polarizer exploiting the semiconductor-metal transition of vanadium dioxide. Operating at a near-infrared wavelength, the device features a SiO2 substrate with VO2 deposited by atomic layer deposition. We demonstrate the design using rigorous coupled wave analysis and show a viable fabrication route. Polarisation-resolved spectral transmission measurements show switching of the extinction ratio from 37.5 (on-state) to 1.6 (off-state). Despite observed deviations between measured and theoretical transmission values, the device shows potential in miniaturized imaging processes, polarization measurements, and ellipsometry.



2:30pm - 2:45pm
ID: 455 / TOM5 S02: 4
TOM 5 Optical Materials

Micro-porous aluminum nitride wick for non-photo-thermal desalination

James Leung, Ji Feng, Luat Vuong

UCRIVERSIDE, United States of America

Aluminum nitride is a white, hydrophilic, high-band-gap ceramic. Here we report on the light-induced evaporation of saltwater through a capillary wick composed of drop-cast microparticles. Saltwater evaporation rates are significantly higher than expected. Our results point to significant potential for this interface-driven approach in solar non-thermal desalination and water separation technologies.



2:45pm - 3:00pm
ID: 446 / TOM5 S02: 5
TOM 5 Optical Materials

Exciton fine structure of a single highly anisotropic CsPbBr3 nanocrystal

Victor Guilloux1, Amal Ghribi2, Kaïs Boujdaria2, Thierry Barisien1, Laurent Legrand1, Emmanuel Lhuillier1, Christophe Testelin1, Maria Chamarro1

1Institut des NanoSciences de Paris, CNRS UMR 7588, Sorbonne Université, F-75005 Paris, France; 22LR01ES15 Laboratoire de Physique des Matériaux: Structure et Propriétés, Faculté des Sciences de Bizerte, Université de Carthage, Bizerte 7021, Tunisia

We measured the photoluminescence (PL) of single CsPbBr3 nanocrystals (NCs) that have a highly anisotropic shape and orthorhombic crystal phase. As the thickness of these NCs is much more smaller than the other two dimensions, they are also called nanoplatelets (NPLs). We obtain PL spectra characterized by doublets separated in energy by about 2 meV in average and showing orthogonal and linearly polarized polar lines. We identified these doublets as the two bright-exciton states of the exciton fine structure contained in the plane of the NPLs. By a comparison between theory and experiments, we were able to obtain fundamental parameters as tetragonal and orthorhombic crystal field. We measured and analysed the time-resolved PL evolution as a function of temperature of small ensemble of NPLs. We thus succeed at framing the experimental value of the bright-dark exciton splitting (5-7meV) that is slightly smaller than the theoretical value.

 
3:30pm - 5:00pmTOM5 S03: Optical materials, synthesis characterization and applications
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Akira Satou, Tohoku University, Japan
 
3:30pm - 4:00pm
Invited
ID: 349 / TOM5 S03: 1
TOM 5 Optical Materials

Polarization-anisotropy of mid-infrared emission properties of Er3+ ions in YAlO3 crystal

Ahmed Nady1, Florent Cassouret2, Pavel Loiko1, Simone Normani1, Alain Braud1, Weidong Chen3, Valentin Petrov3, Dunlu Sun4, Peixiong Zhang5, Bruno Viana2, Ammar Hideur6, Patrice Camy1

1Centre de Recherche sur les Ions, les Matériaux et la Photonique (CIMAP), UMR 6252 CEA-CNRS-ENSICAEN, Université de Caen Normandie, 6 Boulevard Maréchal Juin, 14050 Caen, France; 2Chimie ParisTech, PSL University, CNRS, Institut de Recherche de Chimie Paris, 11 rue Pierre et Marie Curie, 75005 Paris, France; 3Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Max-Born-Str. 2a, 12489 Berlin, Germany; 4Anhui Institute of Optics and Fine Mechanics, Hefei Institutes of Physical Science, Chinese Academy of Sciences, 230031 Hefei, China; 5Department of Optoelectronic Engineering, Jinan University, 510632 Guangzhou, China; 6CORIA UMR6614, CNRS-INSA-Université de Rouen Normandie, Normandie Université, 76801 Saint Etienne du Rouvray, France

We report on a polarization-resolved study of mid-infrared emission properties of Er3+ ions in the orthorhombic YAlO3 crystal. For the 4I11/2 → 4I13/2 transition, σSE reaches 0.20×10-20 cm2 at 2919 nm (for light polarization E || c). Pump-induced polarization switching between the E || b and E || c eigen-states is observed in an 10 at.% Er:YAlO3 laser. Pumped by an Yb-fiber laser at 976 nm, this laser delivers 0.77 W at 2919 nm with a slope efficiency of 31.4% being close to the Stokes limit and a laser threshold of 33 mW.



4:00pm - 4:15pm
ID: 136 / TOM5 S03: 2
TOM 5 Optical Materials

Analysis of the recording of Fibonacci lenses using photopolymers with 3-D diffusion model

Juan Carlos Bravo Francés1,2, Joan Josep Sirvent Verdú1,2, José Carlos García Vázquez1,3, Andrés Pérez Bernabeu1,2, Jaume Colomina Martínez1,2, Roberto Fernández Fernández1,2, Andrés Márquez Ruiz1,2, Sergi Gallego Rico1,2

1Instituto Universitario de Física Aplicada a las Ciencias y las Tecnologías, Universidad de Alicante, Apartado 99, E03080 Alicante, Spain; 2Departamento de Física, Ingeniería de Sistemas y Teoría de la Señal. Universidad de Alicante, Apartado 99, E03080 Alicante, Spain; 3Departamento de Óptica, Farmacología y Anatomía. Universidad de Alicante. Apartado 99, E03080 Alicante, Spain

In the present work, a 3-Dimensional diffusion model is proposed to predict the main properties of Diffractive Optical Elements (DOEs), recorded in photopolymers, including refractive index modulation and the evolution of the transverse intensity distribution. The model enables the selection of appropriate material characteristics based on the intended application of the DOE. Specifically, a PVA/AA photopolymer based on acrylamide is simulated using the proposed model, considering coverplating and index matching systems to mitigate the effects of thickness variation. In order to compare its properties using the suggested model, the simulation focuses on a Fibonacci Lens and the dependece of the intensity by the polymerization rate. Accordingly, axial intensity pattern is represented to prove the bifocal-behaviour of these diffractive lenses.



4:15pm - 4:30pm
ID: 363 / TOM5 S03: 3
TOM 5 Optical Materials

Towards freeform manufacturing of ultra-low expansion glass optics

Samuel Youcef Benketaf

Galatea Laboratory, Switzerland

Ultra-Low-Expansion glass (ULE®) has become an important technological enabler of advanced imaging for astronomy and for extreme-UV lithography. A major limitation though, is that ULE® cannot be poured from the fluid state unlike ZERODUR® which renders costly to produce large and/or complex shapes from it. Beside mirrors, optical components are rarely made of ULE® despite it sharing many properties of pure fused silica glass. Here we explore how femtosecond laser processing combined with laser induced reflow can be used to structure ULE® glass with the goal of producing miniature optical components. To fulfil optical roughness requirements, we adopt a strategy based on first producing elementary shapes, such as cubes or cylinders, that we further topologically transform into sphere, ellipsoids or curved surfaces, using a laser-reflow process. The structural modification of the glass matrix induced by the reflow were investigated using Raman spectroscopy. Our result points to a densification of the glass but no apparent sign of crystallization or devitrification. Furthermore, to understand whether the thermo-mechanical properties were affected or not, the thermal expansion coefficient was estimated using a dilatometry technic based on a pseudo-bimorph micro-cantilevers in a temperature-controlled chamber.



4:30pm - 4:45pm
ID: 377 / TOM5 S03: 4
TOM 5 Optical Materials

Exploration of responsive photonic arrays fabricated by two photon lithography

Jing Qian1, Srikanth Kolagatla2, Iseult Ryan2, Larisa Florea2, Colm Delaney2, A. Louise Bradley1

1School of Physics and AMBER, Trinity College Dublin, College Green, Dublin 2, Ireland; 2School of Chemistry and AMBER, Trinity College Dublin, College Green, Dublin 2, Ireland

Responsive hydrogel photonic structures were fabricated using two-photon lithography. The design versatility of two-photon lithography provides for unprecedented manipulation of transmittance and reflectance spectra, producing distinct structural color. Hydrogel photonic structures have potential for wide range applications, in this instance we demonstrate examples of color transformation, reversible vapor sensing, and pH detection.



4:45pm - 5:00pm
ID: 386 / TOM5 S03: 5
TOM 5 Optical Materials

Probing buried interfaces in SiOxNy thin films via ultrafast acoustics: the role transducing layer thickness

Martina Tauchmanova, Pavel Mokry, Vit Kanclir, Jan Vaclavik, Petra Vesela, Karel Zidek

Institute of Plasma Physics of the Czech Academy of Sciences, Czech Republic

Probing buried interfaces in thin films is a crucial task in many fields, including optical coating. Ultrafast acoustics provide a means to characterize the interfaces by using an acoustic wave localized on the nanometer scale. We provide a brief overview of our thorough study of the interface between SiOxNy thin films and Si substrate by using both single-color and broadband picosecond acoustics. The experiment allows us to track the effect of stoichiometry on the acoustics wave propagation and transition over the layer-substrate interface. To optimize the experiment, we also created simulations to study the effect of optoacoustic layer thickness. We show that the used Ti layer features an optimum thickness between 5-10 nm to reveal details of the interface properties.

 
Date: Wednesday, 13/Sept/2023
8:30am - 10:00amTOM5 S04: Optical materials and lasers
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Patricia Segonds, EOS, France
 
8:30am - 9:00am
Invited
ID: 490 / TOM5 S04: 1
TOM 5 Optical Materials

Crystalline waveguides with carbon nanomaterials for miniaturized pulsed lasers

Ji Eun Bae1,2, Fabian Rotermund2

1CIMAP, CNRS, Université de Caen Normandie, France; 2Department of Physics, KAIST, Korea

This presentation discusses the recent results on miniaturized pulsed solid-state lasers by utilizing femtosecond-laser inscribed crystalline channel waveguides and carbon-nanomaterial-based saturable absorbers. Based on optical characterization and optimization of the optical materials, integrated compact waveguide lasers present diverse pulsed operation regimes from Q-switching to continuous-wave mode-locking. Pulsing mechanism and various parameters in waveguide lasers are investigated to provide a basis for achieving higher performance of novel on-chip ultrafast lasers.



9:00am - 9:15am
ID: 128 / TOM5 S04: 2
TOM 5 Optical Materials

Conductive graphitic wires generation in diamond by means of pulsed Bessel beam micromachining

Akhil Kuriakose1,2, Andrea Chiappini3, Belén Sotillo4, Adam Britel5, Pietro Apra5, Federico Picollo5, Ottavia Jedrkiewicz1

1IFN-CNR, Udr di Como, Via Valleggio 11, 22100 Como, Italy; 2Dipartimento di Scienza e Alta Tecnologia, Università dell’Insubria, Via Valleggio 11, 22100 Como, Italy; 3Istituto di Fotonica e Nanotecnologie (IFN)-CNR, CSMFO and FBK-CMM, Trento, Italy, Italy; 4Department of Materials Physics, Faculty of Physics, Complutense University of Madrid, Plaza de Ciencias 1, 28040, Madrid, Spain; 5Department of Physics and “NIS” Inter-departmental Centre, University of Torino, Via Pietro Giuria 1, 10125, Torino, Italy

We present the fabrication of transverse graphitic microelectrodes in a 500 micrometer thick synthetic diamond bulk by means of pulsed Bessel beams. By suitably placing the elongated focal length of the Bessel beam across the entire sample, the graphitic wires grow from the bottom surface up to the top during multiple shot irradiation. The morphology of the microstructures generated and the micro-Raman spectra are studied

as a function of the laser parameters and the diamond crystal orientation. We show the possibility to generate high conductivity microelectrodes, which are crucial for the application of electric fields or current transport/collection in various chips and detectors.



9:15am - 9:30am
ID: 502 / TOM5 S04: 3
TOM 5 Optical Materials

Innovative selective solar absorber for high vacuum flat panel

Daniela De Luca1,3, Antonio Caldarelli1,2, Eliana Gaudino1,2, Paolo Strazzullo1,2, Marilena Musto1,2, Umar Farooq1,3, Emiliano Di Gennaro1,3, Roberto Russo1

1National Research Council of Italy, Napoli Unit, Institute of Applied Sciences and Intelligent Systems, 80131 Napoli, Italy; 2Industrial Engineering Department, University of Napoli “Federico II”, 80126 Napoli, Italy; 3Physics Department, University of Napoli “Federico II”, 80126 Napoli, Italy

Selective Solar Absorbers (SSAs) are the critical element of high-vacuum flat plate collectors, as these are subject to elevated operating temperatures and thus experience high radiation losses. Here we design and optimize an SSA based on a multilayer design made of HfCx, Si3N4, and SiO2 layers. The structure of the proposed SSA has been optimized to maximize the solar-to-thermal energy conversion efficiency in high vacuum solar thermal panels working at 200 °C, reaching thermal emissivity values much lower than absorbers currently available on the market (<0.02 Vs >0.07) and obtaining unprecedented performances.



9:30am - 9:45am
ID: 375 / TOM5 S04: 4
TOM 5 Optical Materials

Study of the pump dependence of the emission properties of a plasmonic array nanolaser

Mirko Trevisani1, Elizabeth Mendoza Sandoval1,2, Giuseppe Pirruccio2, Tiziana Cesca1, Giovanni Mattei1

1University of Padova, Italy; 2Instituto de Fısica, Universidad Nacional Autonoma de Mexico, Mexico

Lattice plasmon lasers demonstrated to have many degrees of freedom useful to tailor the lasing properties, as the tuning of the morphological properties of the array or the coupling of proper emitters to band edge states of the plasmonic crystal. Here, we present the results of the study of the lasing emission properties of a hexagonal array of aluminum nanoparticles as a function of the pumping conditions. We demonstrate how the geometrical and dynamic features of the pumping system have a significant impact on the lasing properties without affecting the temporal coherence of the emission. Moreover, by combining different pumping systems and studies at different incidence angles, the relationship between nanoarray, dye and pump has been clarified.



9:45am - 10:00am
ID: 415 / TOM5 S04: 5
TOM 5 Optical Materials

Optical Gain and Lasing in PbS Quantum Dots beyond 2 μm

Guy Luke Whitworth1, Mariona Dalmases1, Gerasimos Konstantatos1,2

1Institut de Ciències Fotòniques (ICFO); 2Institució Catalana de Recerca i Estudis Avançats (ICREA)

We present PbS colloidal quantum dots (CQDs) as a promising new gain media for the fabrication of tuneable near- to mid-infrared laser sources. Using distributed feedback (DFB) cavities, we have demonstrated lasing within the telecommunication bands between 1.55 μm – 1.65 μm and have now extended this to gain media beyond 2 μm using large PbS CQDs. We have characterised these dots using transient absorption spectroscopy and amplified spontaneous emission, showing them to have a significantly lower gain threshold than their smaller counterparts (down to ~40 μJ/cm2).

 
3:30pm - 5:00pmTOM5 S05: Optical materials and nonlinear optics
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Tiziana Cesca, University of Padova, Italy
 
3:30pm - 4:00pm
Invited
ID: 170 / TOM5 S05: 1
TOM 5 Optical Materials

Effect of geometry, anisotropy and composition on the third-order optical nonlinearities of multilayer hyperbolic metamaterials

Domenico Genchi, Francesca Dodici, Tiziana Cesca, Giovanni Mattei

University of Padua, Department of Physics and Astronomy, NanoStructures Group (NSG), I-35131, Padova, Italy

Quantum technologies require advanced optical metamaterials whose properties can be tailored and controlled as desired. Hyperbolic metamaterials have great potential for applications in nonlinear nanophotonics, such as all-optical switching, optical limiting, mode-locking and optical sensing. In this work, we show how to obtain strong third-order optical nonlinearities in hyperbolic multilayers exploiting the effect of bulk plasmon polaritons. We demonstrate the tunability of these properties with angle and polarization, and we propose a model to predict them. We evidence the enhancement of the nonlinear response in low-loss metamaterials.



4:00pm - 4:15pm
ID: 517 / TOM5 S05: 2
TOM 5 Optical Materials

First measurements of second-order frequency conversion phase-matching conditions in the new CTAS crystal

Théodore Remark1, Patricia Segonds1, Jérôme Debray1, David Jegouso1, Encarnación G. Víllora2, Kiyoshi Shimamura2, Benoit Boulanger1

1Univ. Grenoble Alpes, CNRS, Institut Néel, 38000 Grenoble, France; 2Research Center for Electronic and Optical Materials, National Institute for Materials Science (NIMS), Tsukuba, 305-0044, Japan

We report that Ca3TaAl3Si2O14 is a positive uniaxial crystal and provides second-order frequency conversion. Indeed, we performed direct measurements of phase-matching conditions for second-harmonic generation and sum-frequency generation up to 3.5 µm. The simultaneous fitting of recorded data provided the Sellmeier equations of the two principal refractive indices and the magnitude of the nonlinear coefficient.



4:15pm - 4:30pm
ID: 259 / TOM5 S05: 3
TOM 5 Optical Materials

Temperature dependence of LiTaO3 refractive index: correction of Sellmeier equation

Safia Mohand Ousaid1, Kai.-H Chang1,2, Lung.-H Peng2, Azzedine Boudrioua1

1Université Sorbonne Paris Nord; 2National Taiwan University

We report a new and more precise Sellmeier equation derived using the quasi-phase-matching curves obtained from the study of the optical parametric generation (OPG) in 1D periodically poled LiTaO3 (1D-PPLT) of different periods at low and high pump power



4:30pm - 4:45pm
ID: 189 / TOM5 S05: 4
TOM 5 Optical Materials

Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires

Mattias Jansson1, Fumitaro Ishikawa2, Weimin M. Chen1, Irina A. Buyanova1

1Department of Physics, Chemistry and Biology, Linköping University, SE-58183 Linköping, Sweden; 2Research center for integrated quantum electronics, Hokkaido University, Sapporo 060-8628, Japan

Photon energy upconversion, i.e. the conversion of several low-energy photons to a photon of higher energy, offers significant potential for nano-optoelectronics and nanophotonics applications. The primary challenge is to achieve high upconversion efficiency and a broad device performance range, enabling effective upconversion even at low excitation power. This study demonstrates that core/shell semiconductor nanowire heterostructures can exhibit upconversion efficiencies exceeding what was previously reported for semiconductor nanostructures even at a low excitation power of 100 mW/cm2, by a two-photon absorption process through conduction band states of the narrow-bandgap nanowire shell region. By engineering the electric-field distribution of the excitation light inside the NWs, upconversion efficiency can be further improved by eight times. This work showcases the effectiveness of the proposed approach in achieving efficient photon upconversion using core/shell NW heterostructures, resulting in some of the highest upconversion efficiencies reported in semiconductor nanostructures. Additionally, it offers design guidelines for enhancing energy upconversion efficiency.



4:45pm - 5:00pm
ID: 501 / TOM5 S05: 5
TOM 5 Optical Materials

Infrared tunable 5%MgO:PPLN OPO pumped by a 1-kHz sub-nanosecond microchip laser

Baptiste Bruneteau1,2, Basile Faure2, Jérôme Debray1, Grégoire Souhaité2, Patricia Segonds1, Hideki Ishizuki3, Takunori Taira3, Benoit Boulanger1

1Université Grenoble Alpes, France; 2Teem Photonics, France; 3IMS, Japan

We built and studied a singly resonant optical parametric oscillator using a 5%MgO:PPLN partial cylinder pumped by a sub-nanosecond microlaser emitting 1064 nm at a repetition rate of 1kHz. It is continuously tunable from 1410 nm up to 4330 nm by rotating the cylinder and a total energy of several micro Joules is emitted with a beam quality factor M² lower than 3.

 
Date: Thursday, 14/Sept/2023
8:30am - 10:00amTOM5 S06: Thin films and surfaces
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Monica Bollani, Institute for photonics and nanotechnologies - CNR, Italy
 
8:30am - 9:00am
Invited
ID: 523 / TOM5 S06: 1
TOM 5 Optical Materials

Advances in pulsed laser deposition for thin film growth for photonic waveguide engineering

Eric Kumi-Barimah

School of Chemical and Process Engineering, University of Leeds, United Kingdom

Recently, pulsed laser deposition has been utilised to fabricate multi-component thin films and embed

dissimilar materials (polymer and glasses) and nanoparticles from rare earth ions doped glasses target. This review

presents the results of ns/fs-PLD fabrication of the rare-earth-doped multicomponent glass thin films onto semiconductor

and silica substrates for engineering optically active optical waveguides for amplifiers, lasers and integrated sensor

applications. We present the results of waveguide analysis by investigating the surface morphology, cross-section, and

the fraction of crystalline phase using electron microscopy and X-ray diffraction. In addition, other complementary

characteristics such as refractive index, photoluminescence and lifetime, and optical gain properties will be presented.



9:00am - 9:15am
ID: 185 / TOM5 S06: 2
TOM 5 Optical Materials

Investigation on subsurface damage patterns in ultrashort pulse laser machining of glass using optical coherence tomography

Samson Frank1, Maria Reichenbächer2, Michael Seiler1, Thomas Arnold3,4, Jens Bliedtner1

1Ernst-Abbe-Hochschule Jena University of Applied Sciences, Fachbereich SciTec, 07745 Jena, Germany; 2Günter-Köhler-Institut für Fügetechnik und Werkstoffprüfung GmbH, 07745 Jena, Germany; 3Leibniz-Institut für Oberflächenmodifizierung e.V., 04318 Leipzig, Germany; 4TU Dresden, Fakultät Maschinenwesen, Institut für Fertigungstechnik, 01062 Dresden, Germany

Ultrashort pulse (USP) laser ablation is gaining popularity as a novel manufacturing technique for brittle materials, enabling the creation of complex freeform shapes that are challenging to produce with conventional optics manufacturing techniques. Freeforms have revolutionized optics manufacturing by providing designers with increased degrees of freedom using non-rotational symmetric components. However, this evolution presents new challenges for manufacturing processes, calling for innovative solutions such as USP ablation. To ensure the industrial viability of areal USP laser machining, it is crucial to not only consider material removal rates but also surface quality and subsurface damage (SSD). Especially for optical applications, harsh quality requirements must be met. This study investigates the SSD patterns of fused silica (FS) and borosilicate glass N-BK7 (BK) processed under different laser wavelengths, beam geometries and processing parameters using high-resolution optical coherence tomography (OCT). It is shown that OCT as non-destructive and 3D evaluation method is well-suited for analysing USP processes. The discovered differences in defect morphology between FS and BK emphasize the importance of selecting appropriate processes and process parameters when working with different materials. Compared to previous studies which used destructive techniques for SSD analysis, OCT revealed higher defects depths of up to 441 µm.



9:15am - 9:30am
ID: 150 / TOM5 S06: 3
TOM 5 Optical Materials

Franck Condon analysis of emission and excitation spectra of fused silica materials

Mariem Guesmi1, Tomas Thor1, Oumayma Taboubi2, Ivana Šeděnková2, Yadu Ram Panthi2, Jiri Pfleger2, Karel Zidek1

1Regional Center for Special Optics and Optoelectronic Systems (TOPTEC), Institute of Plasma Physics of the Czech Academy of Sciences, Za Slovankou 1782/3, 182 00 Prague 8-Liben, Czech Republic; 2Institute of Macromolecular Chemistry, Academy of Sciences of the Czech Republic, 162 06 Prague 6, Czech Republic

Analysis of defects in optical materials is essential for their applicability in cutting-edge optical components. Since fused silica (FS) counts among the most used materials, deep knowledge about the defects in FS is of high importance. These defects have been routinely identified by studying photoluminescence (PL) emission and its analysis via multiple Gaussian bands. Here we present an extended approach based on the Franck-Condon model to study the defects in FS and the connected pathways of charge carrier relaxation. First, we performed the optical characterization of the FS, including optical absorption, photoluminescence (PL) emission and excitation (PLE), and Fourier-transform infrared (FTIR) and Raman spectroscopy (RS). Based on the analysis of the PLE spectra and vibrational frequencies via RS and FTIR, we created a multi-transition Franck-Condon model, which is able to fully reproduce the PL and PLE spectra. Based on the experimental data and the Franck-Condon fit, we discuss two types of oxygen-deficient centres (ODC) present in this fused silica material and their emission pathways.



9:30am - 9:45am
ID: 493 / TOM5 S06: 4
TOM 5 Optical Materials

Stochastic antireflection structures on silicon fabricated by reactive ion etching

David Schmelz1, Thomas Käsebier1, Uwe Zeitner2,3

1Institute of Applied Physics, Abbe Center of Photonics, Friedrich Schiller University Jena, Germany; 2Fraunhofer Institute for Applied Optics and Precision Engineering IOF, Jena, Germany; 3Department of Applied Sciences and Mechatronics, Munich University of Applied Sciences, Munich, Germany

Stochastic Si nanostructures for antireflection (AR) fabricated by reactive ion etching (RIE) are presented for use in different spectral ranges. The lithography-free fabrication enables its application on highly curved surfaces. ALD-coatings of Al2O3 of varying thickness can improve the mechanical stability of such structures while keeping their optical functionality. While typical black silicon structures are suitable for application from VIS to NIR, an RIE-based fabrication process for stochastic AR structures in the longer IR and THz range is presented as well.



9:45am - 10:00am
ID: 458 / TOM5 S06: 5
TOM 5 Optical Materials

Capability and limits of the technology of complex optical interference filters

Antonin Moreau, Cihan Koc, Olivier Hector, Fabien Lemarchand, Frederic Lemarquis, Aude Lereu, Julien Lumeau

Aix-Marseille Univ, CNRS, Centrale Marseille, Institut Fresnel, UMR 7249, 13013 Marseille, France

Over the last 15 years, there have been tremendous progress in the technology of optical interference filters. Nowadays, it is more and more common to fabricate optical interference filters that can combine several tens to several hundreds of layers in order to produce more and more complex optical functions. These progresses are the result of improved multilayer structures modeling and design procedures, the introduction of Virtual Deposition Process, and the development of performant physical vapor deposition machines associated with in-situ optical monitoring. In this paper, we will present actual state-of-the-art of these technologies and some typical examples of filters. We will then present some of the actual challenges and outlook in order to produce more and more performant optical components.

 
3:30pm - 5:00pmTOM6 S04: Entangled states generation
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Kamel Bencheikh, Center for Nanoscience and Technology, France
 
3:30pm - 4:00pm
Invited
ID: 474 / TOM6 S04: 1
TOM 6 Nonlinear and Quantum Optics

Spatially entangled states of light in nonlinear waveguide arrays

Arnault Raymond1, Saverio Francesconi1, José Palomo2, Pascal Filloux1, Martina Morassi3, Aristide Lemaître3, Fabrice Raineri3,4, Maria Amanti1, Sara Ducci1, Florent Baboux1

1Université Paris Cité, France; 2LPENS, Université PSL, France; 3Université Paris-Saclay, CNRS, France; 4Université Côte d’Azur, France

We demonstrate a nonlinear AlGaAs photonic chip generating biphotons with nonclassical spatial correlations. Photon pairs are generated by parametric down conversion in a waveguide array and simultaneously spread through quantum walks along the various waveguides. This concept implements a compact and versatile source of spatially entangled states, operating at room temperature and telecom wavelength, that could serve as a workbench for simulating condensed matter problems on-chip.



4:00pm - 4:15pm
ID: 175 / TOM6 S04: 2
TOM 6 Nonlinear and Quantum Optics

Broadband biphoton generation and polarization splitting in a monolithic AlGaAs chip

Othmane Meskine1, Félicien Appas1,2, Aristide Lemaître3, José Palomo4, Florent Baboux1, Maria I. Amanti1, Sara Ducci1

1Université Paris Cité, CNRS, Laboratoire Matériaux et Phénomènes Quantiques, 75013 Paris, France; 2ICFO - Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Castelldefels (Barcelona) 08860, Spain; 3Université Paris-Saclay, CNRS, Centre de Nanosciences et de Nanotechnologies, 91120, Palaiseau, France; 4Laboratoire de Physique de l’École normale supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris Cité, 75005 Paris, France

Integrated quantum photonics is a key tool towards large scale quantum technologies. In this work we present an AlGaAs-based photonic circuit for the on-chip generation of broadband orthogonally polarized photons and the deterministic separation of the photons into separate spatial modes, facilitating their further use in protocols. We demonstrate that 85% of the pairs are deterministically separated by the chip over a full 60 nm bandwidth and we assess the chip operation in the quantum regime via a Hong-Ou-Mandel experiment displaying a raw visibility of 75.5% over the same full bandwidth.



4:15pm - 4:30pm
ID: 117 / TOM6 S04: 3
TOM 6 Nonlinear and Quantum Optics

Local sampling of the SU(1,1) Wigner function

Nicolas Fabre1, Andrei Klimov2, Gerd Leuchs3,4, Luis Sanchez Soto3,5

1Telecom Paris, France; 2Departamento de Física, Universidad de Guadalajara, 44420 Guadalajara, Jalisco, Mexico; 3Max-Planck-Institut für die Physik des Lichts, 91058 Erlangen, Germany; 4Institut für Optik, Information und Photonik, Friedrich-Alexander-Universität Erlangen-Nürnberg, 91058 Erlangen, Germany; 5Departamento de Óptica, Universidad Complutense, 28040 Madrid, Spain

The Wigner phase-space formulation for systems possessing SU(1,1) symmetry has been defined by Seyfarth et al. [Quantum 4, 317 (2020)] tackling the difficulty in defining a suitable operational definition of the Wigner function. To further investigate this formulation, we propose a non-linear optical setup that incorporates photon-number-resolving detectors, which would enable a direct and comprehensive point-by-point sampling of the SU(1,1) Wigner function. We discuss the visualization of various two-mode quantum states and the effect of the losses in such a detection scheme.



4:30pm - 4:45pm
ID: 160 / TOM6 S04: 4
TOM 6 Nonlinear and Quantum Optics

Making entanglement between photonic Orbital Angular Momenta by Spontaneous Four Wave Mixing in an atomic vapor

Laurence Pruvost, Myrann Abobaker

LCPMR, CNRS, Sorbonne-Université, France

Spontaneous Four Wave Mixing (SFWM) which generates photonic pairs is studied if it is addressed by optical vortices carrying an orbital angular momentum (OAM). We show that the output beams are OAM-correlated and that the entanglement depends on the 4-level scheme used to realize SFWM.

 
5:00pm - 6:30pmTOM6 S05: Nonlinear wave mixing and frequency combs
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Sonia Boscolo, Aston University, United Kingdom
 
5:00pm - 5:15pm
ID: 425 / TOM6 S05: 1
TOM 6 Nonlinear and Quantum Optics

Complex interactions of breathers

Andrey Gelash1, Amin Chabchoub2, Bertrand Kibler1

1Université Bourgogne Franche-Comté, Dijon, France; 2Hakubi Center for Advanced Research, Kyoto University, Kyoto, Japan

We present our recent theoretical and experimental advancements in studying complex multiple nonlinear interactions of coherent solitary wave structures on unstable background -- breathers. We use the focusing one-dimensional nonlinear Schrödinger equation (NLSE) as a theoretical model. First, we describe the nonlinear mutual interactions between a pair of co-propagative breathers called breather molecules. Then with the novel approach of breather interaction management, we adjust the initial positions and phases of several breathers to observe various desired wave states at controllable moments of evolution. Our experiments carried out on a light wave platform with a nearly conservative optical fiber system accurately reproduce the predicted dynamics. In addition, we consider generalizations of the scalar breathers theory to the vector two-component NLSE describing polarized light and show examples of resonance vector breathers transformations.



5:15pm - 5:30pm
ID: 147 / TOM6 S05: 2
TOM 6 Nonlinear and Quantum Optics

Predicting frequency comb structure in nonlinear optical fibre using a neural network

Sonia Boscolo1, John Dudley2, Christophe Finot3

1Aston Institute of Photonic Technologies, Aston University, Birmingham B4 7ET, United Kingdom; 2Université de Franche-Comté, Institut FEMTO-ST, CNRS UMR 6174, Besançon, France; 3Laboratoire Interdisciplinaire CARNOT de Bourgogne- UMR 6303 CNRS - Université de Bourgogne, France

We deploy a neural network to predict the spectro-temporal evolution of simple sinusoidal temporal modulations upon propagation in a nonlinear dispersive fibre. Thanks to the speed of the neural network, we can efficiently scan the input parameter space for the generation of on-demand frequency combs or the occurrence of substantial spectral/temporal focusing.



5:30pm - 5:45pm
ID: 142 / TOM6 S05: 3
TOM 6 Nonlinear and Quantum Optics

Dynamics control in four-wave mixing processes in optical fiber

Anastasiia Sheveleva1, Pierre Colman1, John M. Dudley2, Christophe Finot1

1Laboratoire Interdisciplinaire CARNOT de Bourgogne, UMR 6303 CNRS-Université de Bourgogne, Dijon, France; 2Université de Franche-Comté, Institut FEMTO-ST, CNRS UMR 6174, Besançon, France

A nonlinear interaction of waves in a dispersive medium manifests itself in a four-wave mixing process that can be described as an evolution of waves’ parameters on a phase plane in a form of closed orbits. Here we propose a method to control these trajectories and to switch from one state to another in an optimal manner by implementing an abrupt change of the average power. The method is confirmed experimentally by the reconstruction of a fundamental four-wave mixing dynamics in an idealized model using iterative propagation in a short segment of fiber.



5:45pm - 6:00pm
ID: 508 / TOM6 S05: 4
TOM 6 Nonlinear and Quantum Optics

4-Field spontaneous symmetry breakings in photonic molecules

Alekhya Ghosh1,2, Lewis Hill1,3, Gian-Luca Oppo3, Pascal Del'Haye1,2

1Max Planck Institute for the Science of Light, Germany; 2Department of Physics, Friedrich Alexander University Erlangen-Nuremberg, 91058 Erlangen, Germany; 3SUPA & CNQO, Department of Physics, University of Strathclyde, 107 Rottenrow, Glasgow, G4 0NG, UK

We present in this work a study of 4-field symmetry breakings in two photonic molecule structures consisting of two identical microresonators with distinct coupling arrangements. Mediated by the Kerr-interaction, the systems also display different 2-field symmetry breakings, periodic switching and chaos. The wide range of nonlinear optical dynamics makes the system ideal for all-optical switching, optical memories, telecommunication systems, polarization controllers and integrated photonic sensors.



6:00pm - 6:15pm
ID: 414 / TOM6 S05: 5
TOM 6 Nonlinear and Quantum Optics

Frequency comb atom interferometry

Clément Debavelaere1, Cyrille Solaro1, Pierre Cladé1, Saïda Guellati-Khélifa1,2

1Laboratoire Kastler Brossel, France; 2Conservatoire National des Arts et Métiers

We have implemented of a light pulse atom interferometer based on the diffraction of free-falling atoms of Rubidium by a picosecond frequency-comb laser. We have studied the impact of the pulses' length as well as of the interrogation time on the contrast of the fringes. Our data are well reproduce by a theoretical model based on the effective coupling which depend on the overlap between the pulses and the atoms. This technique, which we demonstrated in the visible spectrum on Rb atoms, paves the way for extending light-pulse interferometry to other spectral regions (deep-UV to X-UV) and therefore to new species, since one can benefit from the high peak intensity of the ultrashort pulses which makes nonlinear frequency conversion in crystals and gas targets more efficient.



6:15pm - 6:30pm
ID: 462 / TOM6 S05: 6
TOM 6 Nonlinear and Quantum Optics

Enhancing THz wave generation in silica nanofibers with Zinc Telluride nonlinear coating

Abderrahim Azzoune1, Sylvie Lebrun2

1Ecole Militaire Polytechnique, Laboratoire Systèmes Lasers, BP17, 16111, Bordj-El-Bahri, Algiers, Algeria; 2Université Paris-Saclay, Institut d’Optique Graduate School, CNRS, Laboratoire Charles Fabry, 91127, Palaiseau, France

This study investigates the use of Zinc Telluride (ZnTe) as a second-order nonlinear coating to enhance THz wave generation in silica nanofibers. Numerical simulations show that ZnTe coatings can significantly improve THz wave generation efficiency due to their large second-order nonlinear susceptibility and high transparency in the THz frequency range. Specifically, we observe a 2000-fold increase in THz wave generation efficiency with a 100nm thickness ZnTe coating compared to an uncoated silica nanofiber.

 
Date: Friday, 15/Sept/2023
8:30am - 10:00amTOM6 S06: Nonlinear multimode fiber optics
Location: Meursault/ Nuit ST-G./Corton
Session Chair: Kamel Bencheikh, Center for Nanoscience and Technology, France
 
8:30am - 9:00am
Invited
ID: 287 / TOM6 S06: 1
TOM 6 Nonlinear and Quantum Optics

Thermalization of light waves in multimode optical fibers: Negative temperatures equilibrium states and the role of disorder

Kilian Baudin1, Josselin Garnier2, Nicolas Berti1, Adrien Fusaro3, Lucas Zanaglia4, Claire Michel4, Valérie Doya4, Katarzyna Krupa5, Guy Millot1, Antonio Picozzi1

1CNRS - Université de Bourgogne, ICB, Dijon, France; 2CMAP, CNRS, Ecole Polytechnique, Institut Polytechnique de Paris, France; 3CEA, DAM, Arpajon, France; 4Université Côte d’Azur, CNRS, Institut de Physique de Nice, Nice, France; 5Institute of Physical Chemistry Polish Academy of Sciences, Warsaw, Poland

Nonlinear random waves exhibit a phenomenon of irreversible thermalization, in analogy with the thermalization of a classical gas system. This irreversible process of thermalization to the Rayleigh-Jeans equilibrium distribution has been recently observed experimentally in multimode optical fibers. Here we discuss a recent progress along two different directions. Firstly, we report the observation of thermalization to negative temperature equilibrium states, in which high-order fiber modes are more populated than low-order modes. Secondly, we analyze the impact of disorder inherent to light propagation in multimode fibers. We identify an unexpected regime in which strong random coupling among non-degenerate modes leads to a nonequilibrium process of thermalization.



9:00am - 9:15am
ID: 364 / TOM6 S06: 2
TOM 6 Nonlinear and Quantum Optics

Full-beam spatial coherence measurements of supercontinuum generation in multimode fibers

Jiaqi Li, Piotr Ryczkowski, Goëry Genty

tampere university, Finland

We study experimentally the spatial coherence across the full spatial beam profile of supercontinuum light generated in both in graded-index and step-index multimode fibers. We observe a decrease of the coherence area with an increase of the injected pump power. Numerical simulations based on linearly polarized modes and mode coupling theory are in good agreement with our experiments and indicate that the decrease of coherence area is strongly related to a change in the modal amplitude distribution.



9:15am - 9:30am
ID: 360 / TOM6 S06: 3
TOM 6 Nonlinear and Quantum Optics

Mid-infrared generation beyond 3.5 μm in a graded-index silica fiber

Karolina Stefańska1,2, Pierre Béjot1, Julien Fatome1, Guy Millot1, Karol Tarnowski2, Bertrand Kibler1

1Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR6303 CNRS-Université de Bourgogne, Dijon, France; 2Department of Optics and Photonics, Wrocław University of Science and Technology, Wrocław, Poland

We present theoretical as well as experimental evidence of far-detuned nonlinear wavelength conversion towards the mid-infrared, namely beyond 3.5 μm, in a few-mode graded-index silica fiber pumped at 1.064 μm. We take into account the full frequency-dependence of the propagation constants, which allows us to obtain excellent agreement of theoretical predictions with experimental observations and provides new and accurate interpretation of intramodal and intermodal four-wave mixing processes in few-mode fibers.



9:30am - 10:00am
Invited
ID: 275 / TOM6 S06: 4
TOM 6 Nonlinear and Quantum Optics

Beam-by-beam Kerr clean-up in multimode optical fibres

Mario Ferraro1,2, Fabio Mangini1, Yann Leventoux3, Alessandro Tonello3, Mario Zitelli1, Yifan Sun1, Sebastien Fevrier3, Katarzyna Krupa4, Denis Kharenko5,6, Stefan Wabnitz1, Vincent Couderc3

1DIET, Sapienza University of Rome, Via Eudossiana 18, 00184 Rome, Italy; 2Department of Physics, University of Calabria, Via P. Bucci, 87069 Rende, Italy; 3XLIM, UMR CNRS 7252, University of Limoges, 123 Avenue A. Thomas, 87060 Limoges, France; 4Institute of Physical Chemistry, Polish Academy of Sciences, Warsaw, Poland; 5Institute of Automation and Electrometry SBRAS, 1 ac. Koptyug ave., Novosibirsk 630090, Russia; 6Novosibirsk State University, Novosibirsk 630090, Russia

We propose and demonstrate the concept of beam-by-beam cleaning in multimode optical fibres, i.e., the increase of the spatial quality of an intense laser beam, induced by a relatively weak, quasi singlemode seed beam. This effect, which relies on the Kerr nonlinearity of the fibre, is quite efficient: a seed beam is capable of providing a bell-shape to a ten times more powerful beam. Our results pave the way for the development of a new class of all-optical switching devices for intense laser beams.

 

 
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